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[ACS Appl. Mater. Interfaces] Enhanced Conductivity and Thermochromic Luminescence in Hydrogen Bond-Stabilized Columnar Liquid Crystals
作者:Bin Mu, Yu Zhao, Xun Li, Xuhong Quan, and Wei Tian*
關鍵字:iquid crystal, discotic columnar mesophase, hydrogen bond, conductivity, luminescence, thermochromic behavior
論文來源:期刊
具體來源:ACS Appl. Mater. Interfaces 2020, 12, 9637-9645
發表時間:2020年

Developing discotic columnar liquid crystals (LCs) with both high electrical conductivity and strong luminescence remains a challenge because the intracolumnar interdisc π-π stacking usually in ordered discotic columnar LCs is essential to generate charge transport pathways but normally detrimental to light emissions. We here present tricyanotristyrylbenzene-based quasi-discotic LCs upon bearing three wedge-shaped alkyl tails for addressing this issue. The resulted columnar materials displayed both high electrical conductivity and strong luminescence, especially for the ones stabilized by multivalent hydrogen-bonding interactions. Besides, an interesting thermochromic luminescence tuning behavior in a smooth manner was observed over a wide wavelength range for the hydrogen bond-stabilized columnar LCs. This study will lead to the future design and application of new multifunctional optoelectronic materials by integrating excellent conductivity and luminescence tuning behaviors.


全文鏈接:

https://dx.doi.org/10.1021/acsami.9b20769

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