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Two Aromatic Rings Coupled a Sulfur-Containing Group to Favor Protein Electron Transfer by Instantaneous Formations of π∴S:π?π:S∴π or π∴π:S?π:π∴S Five-Electron Bindings
來源:陳效華教授個人網站 發布日期:2016-04-04
作者:Weichao Sun, Haisheng Ren, Ye Tao, Dong Xiao, Xin Qin, Li Deng, Mengyao Shao, Jiali Gao*, and Xiaohu
關鍵字:Two Electron Relay; π∴S:π?π:S∴π; π∴π:S?π:π∴S
論文來源:期刊
具體來源:J. Phys. Chem. C, 2015, 119 (17), 9149–9158.
發表時間:2015年
The cooperative interactions among two aromatic rings with a S-containing group are described, which may participate in electron hole transport in proteins. Ab initio calculations reveal the possibility for the formations of the π∴S:π?π:S∴π and π∴π:S?π:π∴S five-electron bindings in the corresponding microsurrounding structures in proteins, both facilitating electron hole transport as efficient relay stations. The relay functionality of these two special structures comes from their low local ionization energies and proper binding energies, which varies with the different aromatic amino acids, S-containing residues, and the arrangements of the same aromatic rings according to the local microsurroundings in proteins.
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